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Top 20 Most Read Articles

May 2009

The 20 articles with the most full-text downloads during the month, in descending order.


A metallic graphene layer adsorbed with lithium

Chih-Kai Yang

Appl. Phys. Lett. 94, 163115 (2009); http://dx.doi.org/10.1063/1.3126008 (3 pages)

Online Publication Date: 24 April 2009

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We found, by density functional calculation, that lithium atoms can be bonded to a graphene layer alternately on both sides by distorting the relative positions of the carbon atoms in the honeycomb lattice. Compared to the recently synthesized graphane by hydrogenation in which each carbon is pulled out of the plane by hydrogen, the carbon is pushed off instead by the attached lithium. And, surprisingly, the counterintuitive structure is a conductor. This should give consequences to its application in lithium storage.
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68.43.-h Chemisorption/physisorption: adsorbates on surfaces
71.15.Nc Total energy and cohesive energy calculations
71.15.Mb Density functional theory, local density approximation, gradient and other corrections

Resonant spin-filtering in cobalt decorated nanotubes

X. Blase and E. R. Margine

Appl. Phys. Lett. 94, 173103 (2009); http://dx.doi.org/10.1063/1.3120553 (3 pages)

Online Publication Date: 28 April 2009

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We study by means of first-principles calculations within the Landauer formalism the transport properties of carbon nanotubes filled with cobalt clusters. We show that in the limit of small cluster sizes, a significant spin polarization of the incoming ππ wave packets can be obtained on a large energy range around the Fermi level. However, in the limit of increasing cluster size, both the spin polarization and total conductance decrease dramatically, suggesting that strategies to limit the diffusion of magnetic adatoms must be found for applications in spintronics.
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73.63.Fg Nanotubes
72.25.-b Spin polarized transport
73.22.-f Electronic structure of nanoscale materials and related systems

Buckling beam micromechanical memory with on-chip readout

D. Roodenburg, J. W. Spronck, H. S. J. van der Zant, and W. J. Venstra

Appl. Phys. Lett. 94, 183501 (2009); http://dx.doi.org/10.1063/1.3129195 (3 pages)

Online Publication Date: 4 May 2009

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We have used double clamped beams to implement a mechanical memory. Compressive stress is generated by resistive heating of the beams and beyond the buckling limit the bistable regime is accessed. Bits are written by applying lateral electrostatic forces. The state of the beam is read out by measuring the capacitance between beam and electrodes. Two ways to implement a mechanical memory are discussed: compensation of initial beam imperfections and snap through of the postbuckled beam. Although significant relaxation effects are observed, both methods prove reliable over thousands of write cycles.
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07.10.Cm Micromechanical devices and systems
85.85.+j Micro- and nano-electromechanical systems (MEMS/NEMS) and devices

Electroluminescent measurement of the internal quantum efficiency of light emitting diodes

Amorette Getty, Elison Matioli, Michael Iza, Claude Weisbuch, and James S. Speck

Appl. Phys. Lett. 94, 181102 (2009); http://dx.doi.org/10.1063/1.3129866 (3 pages)

Online Publication Date: 5 May 2009

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An experimental method is demonstrated for the determination of internal quantum efficiency (IQE) in III-nitride-based light-emitting diodes (LEDs). LED devices surrounded with an optically absorbing material have been fabricated to limit collected light to photons emitted directly from the quantum wells across a known fraction of the recombination area. The emission pattern for this device configuration was modeled to estimate the extraction efficiency. IQE can then be calculated from the measured input current and output power. This method was applied to c-plane InxGa1−xN-based LEDs emitting at 445 nm. Initial measurements estimate an IQE of 43%±1% at a current density of 7.9 A/cm2.
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85.60.Jb Light-emitting devices
78.67.De Quantum wells
85.60.Bt Optoelectronic device characterization, design, and modeling

Solution-processed flexible organic transistors showing very-low subthreshold slope with a bilayer polymeric dielectric on plastic

Zihong Liu, Joon Hak Oh, Mark E. Roberts, Peng Wei, Bipul C. Paul, Masaki Okajima, Yoshio Nishi, and Zhenan Bao

Appl. Phys. Lett. 94, 203301 (2009); http://dx.doi.org/10.1063/1.3133902 (3 pages)

Online Publication Date: 18 May 2009

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We demonstrate low-voltage, solution-processed organic transistors on rough plastic substrates with a carrier mobility over 0.2 cm2/V s, a turn-on voltage of near 0 V, and a record low subthreshold slope of ∼ 80 mV/decade in ambient conditions. These exceptional characteristics are attributed to (1) a device stacking architecture with a conducting polymeric gate and a double layered dielectric composed of low-temperature cross-linked poly(4-vinylphenol), (2) a low interface trap density achieved by modifying the dielectric surface with a phenyl-terminated self-assembled monolayer from 4-phenylbutyltrichlorosilane, and (3) controlled crystallization of a small-molecule organic semiconductor film with favorable charge transport microstructure and a low bulk trap density as deposited by an optimized solution-shearing process. The device performance under different operating voltages was also examined and discussed.
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85.30.Tv Field effect devices

Enhanced quantum efficiency of Ge solar cells by a two-dimensional photonic crystal nanostructured surface

I. Prieto, B. Galiana, P. A. Postigo, C. Algora, L. J. Martínez, and I. Rey-Stolle

Appl. Phys. Lett. 94, 191102 (2009); http://dx.doi.org/10.1063/1.3133348 (3 pages)

Online Publication Date: 11 May 2009

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A single-junction germanium solar cell with a photonic crystal nanostructured surface has been developed. The solar cell comprises a Ge p-n junction and an InGaP window layer. The InGaP window layer has been nanopatterned with an extended photonic crystal structure consisting on a triangular lattice of holes with submicronic sizes. Enhancements of the external quantum efficiency of 22% for a wide range of wavelengths and up to a 46% for specific wavelengths have been measured, which implies an increase in photocurrent between 11% and 22%. A clear correlation with the area of photonic crystal patterned has been observed.
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84.60.Jt Photoelectric conversion
42.70.Qs Photonic bandgap materials

The perfect absorber

E. F. C. Driessen and M. J. A. de Dood

Appl. Phys. Lett. 94, 171109 (2009); http://dx.doi.org/10.1063/1.3126062 (3 pages)

Online Publication Date: 29 April 2009

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We demonstrate that films of very lossy metal or dielectric, with a thickness of only a few nanometers, can absorb almost all incident radiation when illuminated from the substrate side at the critical angle for total internal reflection. The absorption for s-polarized light approaches 100%, while the absorption for p-polarized light vanishes. We demonstrate this effect by measuring the absorption as a function of the angle of incidence at a wavelength of 775 nm in a 4.5 nm thick NbN film with a dielectric constant ϵNbN = −8.2+31.4i. The measured absorption in this film reaches a maximum of 94%. We discuss the design of a near-unity efficiency single-photon detector for s-polarized light that has a broadband absorption coefficient of >90% for wavelengths from 700 to 1600 nm.
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77.55.-g Dielectric thin films
61.46.-w Structure of nanoscale materials
85.60.Gz Photodetectors (including infrared and CCD detectors)
78.20.Ci Optical constants (including refractive index, complex dielectric constant, absorption, reflection and transmission coefficients, emissivity)
77.22.Ch Permittivity (dielectric function)

Organic/inorganic hybrid solar cells with vertically oriented ZnO nanowires

Junpeng Liu, Shanshan Wang, Zuqiang Bian, Meina Shan, and Chunhui Huang

Appl. Phys. Lett. 94, 173107 (2009); http://dx.doi.org/10.1063/1.3126955 (3 pages)

Online Publication Date: 28 April 2009

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Hybrid photovoltaic (PV) devices based on copper-phthalocyanine and fullerene combined with ZnO nanowire array as direct charge transport paths were fabricated. The optimized device with ZnO nanowire has a more than fourfold increase in PV performance than the device without nanowire. The former has an open circuit voltage of 0.46 V, a short circuit current of 3.86 mA/cm2, a fill factor of 0.30, and a power conversion efficiency of 0.53%. The hybrid device based on ZnO nanowires with improved PV performance suggests a way for fabrication of PV device with more exciton dissociation interface area and continuous carrier transport paths.
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84.60.Jt Photoelectric conversion
71.35.-y Excitons and related phenomena
81.07.Pr Organic-inorganic hybrid nanostructures
73.40.Kp III-V semiconductor-to-semiconductor contacts, p-n junctions, and heterojunctions
81.16.Be Chemical synthesis methods
72.20.Fr Low-field transport and mobility; piezoresistance

Toward photonic crystal based spatial filters with wide angle ranges of total transmission

A. E. Serebryannikov, A. Y. Petrov, and Ekmel Ozbay

Appl. Phys. Lett. 94, 181101 (2009); http://dx.doi.org/10.1063/1.3127443 (3 pages)

Online Publication Date: 5 May 2009

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Spatial filters with steep switching between wide ranges of total transmission and total reflection can be obtained by using two-dimensional dielectric photonic crystals, which are a few wavelengths thick. The guidelines for engineering bandpass and bandstop filters are given. The flatness of isofrequency contours that are localized around a periphery point of the first Brillouin zone is a necessary but insufficient condition for the existence of wide angle ranges of total transmission at intermediate and large angles of incidence. Such ranges that are wider than 20° are demonstrated.
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42.79.Ci Filters, zone plates, and polarizers
42.70.Qs Photonic bandgap materials

Gigantic enhancement in response and reset time of ZnO UV nanosensor by utilizing Schottky contact and surface functionalization

Jun Zhou, Yudong Gu, Youfan Hu, Wenjie Mai, Ping-Hung Yeh, Gang Bao, Ashok K. Sood, Dennis L. Polla, and Zhong Lin Wang

Appl. Phys. Lett. 94, 191103 (2009); http://dx.doi.org/10.1063/1.3133358 (3 pages)

Online Publication Date: 11 May 2009

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UV response of ZnO nanowire nanosensor has been studied under ambient condition. By utilizing Schottky contact instead of Ohmic contact in device fabrication, the UV sensitivity of the nanosensor has been improved by four orders of magnitude, and the reset time has been drastically reduced from ∼ 417 to ∼ 0.8 s. By further surface functionalization with function polymers, the reset time has been reduced to ∼ 20 ms even without correcting the electronic response of the measurement system. These results demonstrate an effective approach for building high response and fast reset UV detectors.
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85.85.+j Micro- and nano-electromechanical systems (MEMS/NEMS) and devices
85.60.Gz Photodetectors (including infrared and CCD detectors)
73.30.+y Surface double layers, Schottky barriers, and work functions
07.10.Cm Micromechanical devices and systems

Effect of illumination intensity and temperature on open circuit voltage in organic solar cells

Pankaj Kumar, S. C. Jain, Hemant Kumar, Suresh Chand, and Vikram Kumar

Appl. Phys. Lett. 94, 183505 (2009); http://dx.doi.org/10.1063/1.3129194 (3 pages)

Online Publication Date: 6 May 2009

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The effect of illumination intensity and temperature on open circuit voltage (Voc) in organic photovoltaic devices has been investigated. Voc is observed to saturate at high illumination intensities. The illuminated J-V characteristics at different intensities intersect the dark characteristic at a single point. This intersection point is shown to be equal to the built-in voltage (Vbi) in the sample. A reduction in temperature shows increment in saturated Voc. This increment in saturated Voc is attributed to the variation of Vbi with temperature. A model has been presented that explains the observed behavior of Vbi at different temperatures.
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84.60.Jt Photoelectric conversion
85.60.-q Optoelectronic devices

The grain boundary related p-type conductivity in ZnO films prepared by ultrasonic spray pyrolysis

Bin Wang, Jiahua Min, Yue Zhao, Wenbin Sang, and Changjun Wang

Appl. Phys. Lett. 94, 192101 (2009); http://dx.doi.org/10.1063/1.3134486 (3 pages)

Online Publication Date: 11 May 2009

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Intrinsic p-type ZnO thin film was fabricated on sapphire substrate by ultrasonic spray pyrolysis, the p-type ZnO film is achieved using O2 as the carrier gas, with a resistivity of 2.18 Ω cm−1, a carrier concentration of 1.10×1016 cm−3, and a high Hall mobility of 261 cm2/V s. The scanning capacitance microscopy images and annealing the p-type ZnO indicate that the absorbed oxygen in the grain boundary (GB) aroused the p-type conductivity, and the high Hall mobility of the p-type ZnO film own to the quasi-two-dimensional hole gas, which was induced by the negatively charged interface states in the GBs.
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73.61.Ga II-VI semiconductors
61.72.Cc Kinetics of defect formation and annealing
61.72.Mm Grain and twin boundaries
73.50.Jt Galvanomagnetic and other magnetotransport effects (including thermomagnetic effects)
68.55.ag Semiconductors

High field-effect mobility pentacene thin-film transistors with nanoparticle polymer composite/polymer bilayer insulators

Yunseok Jang, Wi Hyoung Lee, Yeong Don Park, Donghoon Kwak, Jeong Ho Cho, and Kilwon Cho

Appl. Phys. Lett. 94, 183301 (2009); http://dx.doi.org/10.1063/1.3124660 (3 pages)

Online Publication Date: 5 May 2009

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High field-effect mobility organic thin-film transistors with nanoparticle polymer composite/polymer bilayer insulators were fabricated. A device composed of a polyvinylphenol (PVP) insulator filled with barium strontium titanate (BST) nanoparticles and coated with a thin polystyrene film was found to exhibit a field-effect mobility (1.2 cm2 V−1 s−1 for a pentacene device) and a field-induced current that are superior to those of devices with only a PVP insulator or a BST-filled PVP insulator. These improvements in the performance are due to an increase in the capacitance and a reduction in the interface roughness of the insulator.
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85.30.Tv Field effect devices
68.35.Ct Interface structure and roughness

Enhancement of light absorption in a quantum well by surface plasmon polariton

J. B. Khurgin and G. Sun

Appl. Phys. Lett. 94, 191106 (2009); http://dx.doi.org/10.1063/1.3137186 (3 pages)

Online Publication Date: 14 May 2009

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We investigate analytically the degree to which the absorption of light in a single quantum well can be enhanced in the proximity of a structured metallic surface and show that the wavelength at which the maximum enhancement of about one order of magnitude is attained depends on metal loss and the initial absorption in a quantum well.
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42.25.Bs Wave propagation, transmission and absorption
78.67.De Quantum wells
73.20.Mf Collective excitations (including excitons, polarons, plasmons and other charge-density excitations)

Resistive switching in nanostructured thin films

H. Silva, H. L. Gomes, Yu. G. Pogorelov, P. Stallinga, D. M. de Leeuw, J. P. Araujo, J. B. Sousa, S. C. J. Meskers, G. Kakazei, S. Cardoso, and P. P. Freitas

Appl. Phys. Lett. 94, 202107 (2009); http://dx.doi.org/10.1063/1.3134484 (3 pages)

Online Publication Date: 20 May 2009

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Planar capacitor structures based on granular films composed of nanometric ferromagnetic grains embedded in an insulating Al2O3 matrix can switch between a high-conductance and a low-conductance state. The switching properties are induced by a forming process. The ON/OFF resistance ratio is as high as 104 under an electrical field of only 15 kV/m. This resistive switching is accompanied by a capacitive switching between two well-defined voltage-independent states, a behavior that is not readily explained by the filamentary type of conduction.
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73.63.Bd Nanocrystalline materials

Many-body effects on terahertz quantum well detectors

X. G. Guo, Z. Y. Tan, J. C. Cao, and H. C. Liu

Appl. Phys. Lett. 94, 201101 (2009); http://dx.doi.org/10.1063/1.3134485 (3 pages)

Online Publication Date: 19 May 2009

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Many-body effects have been investigated in the design of terahertz quantum well photon detectors. A large discrepancy between the theoretical and experimental photoresponse peak positions exist without considering the many-body interactions. The calculated results agree with the experimental data quantitatively with including the exchange-correlation and depolarization effects within the local density approximation. Our numerical results show that it is a must to consider the many-body interactions for designing the quantum well detectors for the terahertz region.
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07.57.Pt Submillimeter wave, microwave and radiowave spectrometers; magnetic resonance spectrometers, auxiliary equipment, and techniques
85.35.Be Quantum well devices (quantum dots, quantum wires, etc.)

Auger recombination rates in nitrides from first principles

Kris T. Delaney, Patrick Rinke, and Chris G. Van de Walle

Appl. Phys. Lett. 94, 191109 (2009); http://dx.doi.org/10.1063/1.3133359 (3 pages)

Online Publication Date: 15 May 2009

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We report Auger recombination rates for wurtzite InGaN calculated from first-principles density-functional and many-body-perturbation theory. Two different mechanisms are examined—inter- and intra-band recombination—that affect different parts of the emission spectrum. In the blue to green spectral region and at room temperature the Auger coefficient can be as large as 2×10−30 cm6 s−1; in the infrared it is even larger. Since Auger recombination scales with the cubic power of the free-carrier concentration it becomes an important nonradiative loss mechanism at high current densities. Our results indicate that Auger recombination may be responsible for the loss of quantum efficiency that affects InGaN-based light emitters.
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79.20.Fv Electron impact: Auger emission
71.20.Nr Semiconductor compounds
72.20.Jv Charge carriers: generation, recombination, lifetime, and trapping
71.15.Mb Density functional theory, local density approximation, gradient and other corrections
72.80.Ey III-V and II-VI semiconductors

All-polymer solar cells based on a blend of poly[3-(10-n-octyl-3-phenothiazine-vinylene)thiophene-co-2,5-thiophene] and poly[1,4-dioctyloxyl-p-2,5-dicyanophenylenevinylene]

Guangyi Sang, Yingping Zou, Yu Huang, Guangjin Zhao, Yi Yang, and Yongfang Li

Appl. Phys. Lett. 94, 193302 (2009); http://dx.doi.org/10.1063/1.3134490 (3 pages)

Online Publication Date: 12 May 2009

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We report all-polymer solar cells (PSCs) based on a polymer blend of poly[3-(10-n-octyl-3-phenothiazine-vinylene)thiophene-co-2,5-thiophene] as donor and poly[1,4-dioctyloxyl-p-2,5-dicyanophenylenevinylene] as acceptor. Strong photoluminescence quenching is observed in the polymer blend indicating the photoinduced charge transfer occurs between the two polymers. The power conversion efficiency of the PSC was improved from 0.41% to 0.8% after 120 °C postannealing, under the illumination of AM 1.5, 100 mW/cm2. We attribute the improved efficiency to better morphological features of the photoactive layer after thermal annealing.
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84.60.Jt Photoelectric conversion

Graphene nanoribbon as a negative differential resistance device

Hao Ren, Qun-Xiang Li, Yi Luo, and Jinlong Yang

Appl. Phys. Lett. 94, 173110 (2009); http://dx.doi.org/10.1063/1.3126451 (3 pages)

Online Publication Date: 29 April 2009

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We present a theoretical study on electronic structure and elastic transport properties of armchair graphene nanoribbon based junctions by using density functional theory calculations and nonequilibrium Green’s function technique. The I-V characteristics of various junctions are examined, which all exhibit robust negative differential resistance (NDR) phenomena. It is found that such NDR behaviors originate from the interaction between the narrow density of states of the doped leads and the discrete states in the scattering region.
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71.20.Tx Fullerenes and related materials; intercalation compounds
73.63.Fg Nanotubes
71.15.Mb Density functional theory, local density approximation, gradient and other corrections
72.20.Ht High-field and nonlinear effects
71.55.Cn Elemental semiconductors
73.63.Rt Nanoscale contacts

Surface plasmon resonances of optical antenna atomic force microscope tips

Yanshu Zou, Paul Steinvurzel, Tian Yang, and Kenneth B. Crozier

Appl. Phys. Lett. 94, 171107 (2009); http://dx.doi.org/10.1063/1.3116145 (3 pages)

Online Publication Date: 29 April 2009

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A method for fabricating optical antennas on atomic force microscope probes using focused ion beam modification is described. We numerically demonstrate that these optical antenna probes provide a large near field intensity enhancement when illuminated at their resonant wavelengths. We experimentally measure the plasmon resonant wavelengths of probes with various lengths. Both simulation and experiment indicate that the resonant wavelength redshifts with increasing antenna length. We anticipate that the optical antenna tips could be used for mapping the field distributions of nanophotonic devices or for high spatial resolution spectroscopy.
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07.79.Lh Atomic force microscopes
73.20.Mf Collective excitations (including excitons, polarons, plasmons and other charge-density excitations)
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