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Top 20 Most Read Articles

June 2012

The 20 articles with the most full-text downloads during the month, in descending order.


Luminescence decay in disordered low‐dimensional semiconductors

X. Chen, B. Henderson, and K. P. O’Donnell

Appl. Phys. Lett. 60, 2672 (1992); http://dx.doi.org/10.1063/1.106891 (3 pages)

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The luminescence decay of excitons in disordered low‐dimensional semiconductors with quantum confinement is shown experimentally to be characterized by a nonexponential profile and an absence of spectral diffusion. We are able to describe this luminescence as a hopping‐assisted recombination using the correlation function approach to nondispersive transport developed by H. Scher, M. F. Shlesinger, and J. T. Bendler [Phys. Today 41, 26 (1991)]. We suggest a simple derivation of analytical functions which accurately describe the anomalous luminescence decays of disordered II‐VI superlattices and of porous silicon, and show that this model includes exponential and Kohlrausch [Pogg. Ann. Phys. 119, 352 (1863)] (stretched‐exponential) relaxations as special cases.
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78.66.-w Optical properties of specific thin films
78.67.-n Optical properties of low-dimensional, mesoscopic, and nanoscale materials and structures
78.47.-p Spectroscopy of solid state dynamics
78.55.-m Photoluminescence, properties and materials

Photo-origami—Bending and folding polymers with light

Jennie Ryu, Matteo D’Amato, Xiaodong Cui, Kevin N. Long, H. Jerry Qi, and Martin L. Dunn

Appl. Phys. Lett. 100, 161908 (2012); http://dx.doi.org/10.1063/1.3700719 (5 pages)

Online Publication Date: 20 April 2012

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Photo-origami uses the dynamic control of the molecular architecture of a polymer by a combination of mechanical and non-contact optical stimuli to design and program spatially and temporally variable mechanical and optical fields into a material. The fields are essentially actuators, embedded in the material at molecular resolution, designed to enable controllable, sequenced, macroscopic bending and folding to create three-dimensional material structures. Here, we demonstrate, through a combination of theory, simulation-based design, synthesis, and experiment, the operative phenomena and capabilities of photo-origami that highlight its potential as a powerful, and potentially manufacturable, approach to create three-dimensional material structures.
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81.40.Lm Deformation, plasticity, and creep
61.41.+e Polymers, elastomers, and plastics
62.20.fg Shape-memory effect; yield stress; superelasticity

Coupling between quantum Hall state and electromechanics in suspended graphene resonator

Vibhor Singh, Bushra Irfan, Ganesh Subramanian, Hari S. Solanki, Shamashis Sengupta, Sudipta Dubey, Anil Kumar, S. Ramakrishnan, and Mandar M. Deshmukh

Appl. Phys. Lett. 100, 233103 (2012); http://dx.doi.org/10.1063/1.3703763 (4 pages)

Online Publication Date: 4 June 2012

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Using graphene resonator, we perform electromechanical measurements in quantum Hall regime to probe the coupling between a quantum Hall (QH) system and its mechanical motion. Mechanically perturbing the QH state through resonance modifies the DC resistance of the system and results in a Fano-lineshape due to electronic interference. Magnetization of the system modifies the resonator’s equilibrium position and effective stiffness leading to changes in resonant frequency. Our experiments show that there is an intimate coupling between the quantum Hall state and mechanics—electron transport is affected by physical motion and in turn the magnetization modifies the electromechanical response.
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81.07.Oj Nanoelectromechanical systems (NEMS)
85.85.+j Micro- and nano-electromechanical systems (MEMS/NEMS) and devices

Experimental isolation of degradation mechanisms in capacitive microelectromechanical switches

Z. Olszewski, R. Houlihan, C. Ryan, C. O’Mahony, and R. Duane

Appl. Phys. Lett. 100, 233505 (2012); http://dx.doi.org/10.1063/1.4726116 (4 pages)

Online Publication Date: 6 June 2012

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DC and bipolar voltage stresses are used to isolate mechanical degradation of the movable electrode from charging mechanism in microelectromechanical capacitive switches. Switches with different metals as the movable electrode were investigated. In titanium switches, a shift in the pull-in voltages is observed after dc stressing whereas no shift occurs after the bipolar stressing, which is to be expected from charging theory. On switches with similar dielectric but made of aluminium, the narrowing effect occurs regardless if dc or bipolar stressing is used, which indicates the mechanical degradation as the mechanism responsible.
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84.32.Dd Connectors, relays, and switches
85.85.+j Micro- and nano-electromechanical systems (MEMS/NEMS) and devices

Continuous-wave terahertz system with a 60 dB dynamic range

I. S. Gregory, W. R. Tribe, C. Baker, B. E. Cole, M. J. Evans, L. Spencer, M. Pepper, and M. Missous

Appl. Phys. Lett. 86, 204104 (2005); http://dx.doi.org/10.1063/1.1935032 (3 pages)

Online Publication Date: 13 May 2005

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We have developed a high-performance continuous-wave terahertz imaging system based on photomixing. The emitter and detector are driven by compact, unstabilized, single-mode diode lasers. The all-optoelectronic, homodyne detection scheme yields both amplitude and phase information, and with careful optimization and matching of both emitter and receiver, a 60 dB dynamic range, at 0.53 THz, can be routinely achieved. This replicates the performance of established pulsed THz imagers at this frequency.
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84.40.-x Radiowave and microwave (including millimeter wave) technology
07.57.-c Infrared, submillimeter wave, microwave and radiowave instruments and equipment
85.60.-q Optoelectronic devices
85.60.Gz Photodetectors (including infrared and CCD detectors)

Novel millimeter‐wave near‐field resistivity microscope

Michael Golosovsky and Dan Davidov

Appl. Phys. Lett. 68, 1579 (1996); http://dx.doi.org/10.1063/1.116685 (3 pages)

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We demonstrate a technique for contactless mapping of resistivity or dielectric constant of surfaces and films with a spatial resolution better than 100 μm. This technique may be used for the nondestructive testing of semiconducting wafers, conducting polymers, oxide superconductors, and printed circuits. The principle of operation consists of the scanning of a tiny millimeter‐wave antenna at a very small height above an inhomogeneous conducting surface and measuring the intensity and phase of the reflected (transmitted) wave. We use a specially designed resonant slit antenna and achieve subwavelength spatial resolution of λ/50. © 1996 American Institute of Physics.
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68.37.Ef Scanning tunneling microscopy (including chemistry induced with STM)
68.37.Ps Atomic force microscopy (AFM)
68.37.Rt Magnetic force microscopy (MFM)
68.37.Uv Near-field scanning microscopy and spectroscopy
85.30.De Semiconductor-device characterization, design, and modeling

Influence of polarity on carrier transport in semipolar (20math) and (20math1) multiple-quantum-well light-emitting diodes

Yoshinobu Kawaguchi, Chia-Yen Huang, Yuh-Renn Wu, Qimin Yan, Chih-Chien Pan, Yuji Zhao, Shinichi Tanaka, Kenji Fujito, Daniel Feezell, Chris G. Van de Walle, Steven P. DenBaars, and Shuji Nakamura

Appl. Phys. Lett. 100, 231110 (2012); http://dx.doi.org/10.1063/1.4726106 (4 pages)

Online Publication Date: 6 June 2012

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We investigate the influence of polarity on carrier transport in single-quantum-well and multiple-quantum-well (MQW) light-emitting diodes (LEDs) grown on the semipolar (20math1) and (20math) orientations of free-standing GaN. For semipolar MQW LEDs with the opposite polarity to conventional Ga-polar c-plane LEDs, the polarization-related electric field in the QWs results in an additional energy barrier for carriers to escape the QWs. We show that semipolar (20math) MQW LEDs with the same polarity to Ga-polar c-plane LEDs have a more uniform carrier distribution and lower forward voltage than (20math1) MQW LEDs.
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85.60.Jb Light-emitting devices
85.35.Be Quantum well devices (quantum dots, quantum wires, etc.)

Semiconductor nanowires for highly sensitive, room-temperature detection of terahertz quantum cascade laser emission

Miriam S. Vitiello, Leonardo Viti, Lorenzo Romeo, Daniele Ercolani, G. Scalari, J. Faist, F. Beltram, L. Sorba, and A. Tredicucci

Appl. Phys. Lett. 100, 241101 (2012); http://dx.doi.org/10.1063/1.4724309 (3 pages)

Online Publication Date: 11 June 2012

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We report on the development of nanowire-based field-effect transistors operating as high sensitivity terahertz (THz) detectors. By feeding the 1.5 THz radiation field of a quantum cascade laser (QCL) at the gate-source electrodes with a wide band dipole antenna, we record a photovoltage signal corresponding to responsivity values >10 V/W, with impressive noise equivalent power levels <6 × 10−11 W/√Hz at room temperature and a wide modulation bandwidth. The potential scalability to even higher frequencies and the technological feasibility of realizing multi-pixel arrays coupled with QCL sources make the proposed technology highly competitive for a future generation of THz detection systems.
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42.55.Px Semiconductor lasers; laser diodes
42.60.By Design of specific laser systems
84.40.-x Radiowave and microwave (including millimeter wave) technology
85.30.Tv Field effect devices
07.57.Pt Submillimeter wave, microwave and radiowave spectrometers; magnetic resonance spectrometers, auxiliary equipment, and techniques

Kelvin probe force microscopy

M. Nonnenmacher, M. P. O’Boyle, and H. K. Wickramasinghe

Appl. Phys. Lett. 58, 2921 (1991); http://dx.doi.org/10.1063/1.105227 (3 pages)

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Measurements of the contact potential difference between different materials have been performed for the first time using scanning force microscopy. The instrument has a high resolution for both the contact potential difference (better than 0.1 mV) and the lateral dimension (<50 nm) and allows the simultaneous imaging of topography and contact potential difference. Images of gold, platinum, and palladium surfaces, taken in air, show a large contrast in the contact potential difference and demonstrate the basic concept.
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73.40.Cg Contact resistance, contact potential
07.79.Cz Scanning tunneling microscopes
61.05.-a Techniques for structure determination

Silicon-based reproducible and active surface-enhanced Raman scattering substrates for sensitive, specific, and multiplex DNA detection

Z. Y. Jiang, X. X. Jiang, S. Su, X. P. Wei, S. T. Lee, and Y. He

Appl. Phys. Lett. 100, 203104 (2012); http://dx.doi.org/10.1063/1.3701731 (4 pages)

Online Publication Date: 14 May 2012

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Silicon-based active and reproducible surface-enhanced Raman scattering (SERS) substrate, i.e., silver nanoparticles decorated-silicon wafers (AgNPs@Si), is employed for constructing high-performance sensors. Significantly, the AgNPs@Si, facilely prepared via in situ AgNPs growth on silicon wafers, features excellent SERS reproducibility and high enhancement factor. Our experiment further demonstrates such resultant silicon-based SERS substrate is efficacious for multiplex, sensitive, and specific DNA detection. In particular, single-base mismatched DNA with low concentrations is readily discriminated by using the AgNPs@Si. Moreover, the silicon-based sensor exhibits adequate multiplexing capacity, enabling unambiguous identification of the dual-target DNA detection.
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87.80.Dj Spectroscopies
87.14.gk DNA
87.15.M- Spectra of biomolecules

Crack-free InGaN multiple quantum wells light-emitting diodes structures transferred from Si (111) substrate onto electroplating copper submount with embedded electrodes

Tufu Chen, Yunqian Wang, Peng Xiang, Ruihong Luo, Minggang Liu, Weimin Yang, Yuan Ren, Zhiyuan He, Yibin Yang, Weijie Chen, Xiaorong Zhang, Zhisheng Wu, Yang Liu, and Baijun Zhang

Appl. Phys. Lett. 100, 241112 (2012); http://dx.doi.org/10.1063/1.4729414 (4 pages)

Online Publication Date: 14 June 2012

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Crack-free InGaN multiple quantum wells (MQWs) light-emitting diodes with embedded electrode structures (EE-LEDs) were transferred from Si (111) substrate onto the electroplating copper submount. Crystalline quality was investigated by the high resolution x-ray diffraction (HR-XRD) measurement, in which no obvious deteriorations were found in the MQWs structure after the LEDs transferred from silicon substrate onto copper except for a partial residual strain relaxation in the film. The strain relaxation after silicon removal leads to a reduction in quantum confined stark effect (QCSE), which results in the enhancement of internal quantum efficiency (IQE). In comparison to the conventional LEDs on silicon substrate, the light output of the EE-LEDs on copper was enhanced by 122% at an injection current of 350 mA. Besides the enhancement of IQE, the improvement is also attributed to the following factors: the removal of the absorptive substrate, the inserting of the metal reflector between the EE-LEDs structure and the copper submount, the elimination of the electrode-shading, and the rough surface of the exposed AlN buffer layer.
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85.60.Jb Light-emitting devices
42.79.Kr Display devices, liquid-crystal devices
82.45.Qr Electrodeposition and electrodissolution
85.35.Be Quantum well devices (quantum dots, quantum wires, etc.)

Very high open-circuit voltage of 5.89 V in organic solar cells with 10-fold-tandem structure

Ye Zou, Zhenbo Deng, William J. Potscavage, Masaya Hirade, Yanqiong Zheng, and Chihaya Adachi

Appl. Phys. Lett. 100, 243302 (2012); http://dx.doi.org/10.1063/1.4729009 (4 pages)

Online Publication Date: 12 June 2012

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Organic solar cells (OSCs) based on chloroaluminum phthalocyanine (ClAlPc) as donor and fullerene C60 as acceptor with a multi-tandem structure were fabricated. We demonstrated very high open-circuit voltage (VOC) and enhanced power conversion efficiency (PCE) for the multi-tandem OSCs. Using a fivefold structure, we obtained PCE of 2.49% with a VOC of 3.50 V, in comparison with PCE of ∼2% and VOC of 0.72–0.81 V for the single device. We also fabricated a tenfold-stacked OSC showing an extremely high VOC of 5.89 V. The multi-tandem OSCs with very high VOC have great potential for applications in limited-area low-power electronics.
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88.40.jr Organic photovoltaics
88.40.hj Efficiency and performance of solar cells

Mechanism of non-metal catalytic growth of graphene on silicon

Guo Hong, Qi-Hui Wu, Jianguo Ren, and Shuit-Tong Lee

Appl. Phys. Lett. 100, 231604 (2012); http://dx.doi.org/10.1063/1.4726114 (5 pages)

Online Publication Date: 6 June 2012

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Compared to preparation on metal substrates, graphene synthesis on non-metal surfaces is highly desirable to avoid the deleterious metallic effects in fabrication of electronic devices. However, study of graphene growth mechanism on non-metal surfaces is rare and little understood. Here, we report that few-layers graphene films can be grown directly on silicon-on-insulator surface. Furthermore, the graphene growth mechanism on non-metal surfaces is proposed as a surface reaction, adsorption, decomposition, and accumulation process.
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81.15.Gh Chemical vapor deposition (including plasma-enhanced CVD, MOCVD, ALD, etc.)
82.65.+r Surface and interface chemistry; heterogeneous catalysis at surfaces
64.75.Bc Solubility
81.05.ue Graphene
68.43.Mn Adsorption kinetics

Graphene/ZnO nanowire/graphene vertical structure based fast-response ultraviolet photodetector

Xue-Wen Fu, Zhi-Min Liao, Yang-Bo Zhou, Han-Chun Wu, Ya-Qing Bie, Jun Xu, and Da-Peng Yu

Appl. Phys. Lett. 100, 223114 (2012); http://dx.doi.org/10.1063/1.4724208 (4 pages)

Online Publication Date: 1 June 2012

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We report the high performance vertical ultraviolet (UV) photodetectors based on single ZnO nanowire (NW) sandwiched between two graphene sheets. The photocurrent on-off ratio, rising time, and recovery speed of our UV detectors are 8 × 102, 0.7 s, and 0.5 s, respectively, which are significantly improved compared to the conventional ZnO NWs photodetectors. The improved performance is attributed to the existence of Schottky barriers between ZnO NW and graphene electrodes. The graphene/ZnO NW/graphene vertical sandwiched structures may be promising candidates for integrated optoelectronic sensor devices.
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85.60.Gz Photodetectors (including infrared and CCD detectors)

Electrically pumped wavelength-tunable blue random lasing from CdZnO films on silicon

Ye Tian, Xiangyang Ma, Lu Jin, Dongsheng Li, and Deren Yang

Appl. Phys. Lett. 100, 231101 (2012); http://dx.doi.org/10.1063/1.4725486 (4 pages)

Online Publication Date: 4 June 2012

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Electrically pumped lasing actions from the metastable CdZnO films have hardly been achieved as yet. Herein, we have demonstrated electrically pumped wavelength-tunable blue random lasing from the hexagonal CdZnO films with different Cd contents, with central wavelength changing from ∼490 to 425 nm. The devices based on the metal-insulator-semiconductor structures of Au/SiO2/CdZnO on silicon substrates are constructed for electrical pumping of the CdZnO films. The insulator layers of SiO2 onto the CdZnO films in the devices should be annealed at sufficiently low temperature such as 400 °C so that the CdZnO films can be kept their integrity in terms of near-band-edge emissions.
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42.55.Rz Doped-insulator lasers and other solid state lasers
42.60.Fc Modulation, tuning, and mode locking

Vacuum nanoelectronics: Back to the future?—Gate insulated nanoscale vacuum channel transistor

Jin-Woo Han, Jae Sub Oh, and M. Meyyappan

Appl. Phys. Lett. 100, 213505 (2012); http://dx.doi.org/10.1063/1.4717751 (4 pages)

Online Publication Date: 23 May 2012

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A gate-insulated vacuum channel transistor was fabricated using standard silicon semiconductor processing. Advantages of the vacuum tube and transistor are combined here by nanofabrication. A photoresist ashing technique enabled the nanogap separation of the emitter and the collector, thus allowing operation at less than 10 V. A cut-off frequency fT of 0.46 THz has been obtained. The nanoscale vacuum tubes can provide high frequency/power output while satisfying the metrics of lightness, cost, lifetime, and stability at harsh conditions, and the operation voltage can be decreased comparable to the modern semiconductor devices.
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85.30.Tv Field effect devices
85.35.-p Nanoelectronic devices

Controlled addressing of quantum dots by nanowire plasmons

Christian Gruber, Primoz Kusar, Andreas Hohenau, and Joachim R. Krenn

Appl. Phys. Lett. 100, 231102 (2012); http://dx.doi.org/10.1063/1.4725490 (3 pages)

Online Publication Date: 4 June 2012

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We demonstrate optical near field coupling of small quantum dot (QD) ensembles and surface plasmons propagating along a silver nanowire. The nanowire fabrication and the aligned QD deposition close to one nanowire end rely on a two-step electron beam lithography procedure. We observe both the addressing of QDs by plasmons and the excitation of plasmonic nanowire modes by QDs. We use the fluorescence signals to quantify the QD/plasmon coupling and show that part of the plasmon-induced QD fluorescence couples back to plasmonic modes.
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78.67.Hc Quantum dots
81.16.Nd Micro- and nanolithography
78.55.-m Photoluminescence, properties and materials
73.20.Mf Collective excitations (including excitons, polarons, plasmons and other charge-density excitations)
78.67.Uh Nanowires
81.07.Gf Nanowires

Efficient single-photon extraction from quantum-dots embedded in GaAs micro-pyramids

Daniel Rülke, Daniel M. Schaadt, Heinz Kalt, and Michael Hetterich

Appl. Phys. Lett. 100, 251101 (2012); http://dx.doi.org/10.1063/1.4729482 (4 pages)

Online Publication Date: 18 June 2012

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We demonstrate an easy method to fabricate efficient single-photon sources based on In(Ga)As quantum-dots embedded in reversed GaAs micro-pyramids. It relies on a single wet-chemical etching step utilizing an AlAs sacrificial layer. Due to the pyramidal shape of the cavities, we have been able to separate a small number of quantum-dots from the self-assembled ensemble and improve the extraction efficiency for single photons. The latter is predicted by finite difference time domain and finite elements method simulations to be about 80%–90% over a broad spectral range of 40 nm. Single-photon emission has been proven experimentally by means of auto-correlation measurements.
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81.07.Ta Quantum dots
02.70.Dh Finite-element and Galerkin methods
81.16.Dn Self-assembly
81.05.Ea III-V semiconductors

Phase separation of co-evaporated ZnPc:C60 blend film for highly efficient organic photovoltaics

Ying Zhou, Tetsuya Taima, Tetsuhiko Miyadera, Toshihiro Yamanari, Michinori Kitamura, Kazuhiro Nakatsu, and Yuji Yoshida

Appl. Phys. Lett. 100, 233302 (2012); http://dx.doi.org/10.1063/1.4726118 (5 pages)

Online Publication Date: 5 June 2012

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We demonstrate phase separation of co-evaporated zinc phthalocyanine (ZnPc) and fullerene (C60) for efficient organic photovoltaic cells. With introducing a poly(3,4-ethylenedioxythiophene):poly(styrene sulfonate) film and a crystalline copper iodide film on indium tin oxide, 20-nm-thick ZnPc film adopts a lying-down crystalline geometry with grain sizes of about 50 nm. This surface distributed with strong interaction areas and weak interaction areas enables the selective growth of ZnPc and C60 molecules during following co-evaporation, which not only results in a phase separation but also improve the crystalline growth of C60. This blend film greatly enhances the efficiencies in photocurrent generation and carrier transport, resulting in a high power conversion efficiency of 4.56% under 1 sun.
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68.35.bp Fullerenes
61.48.-c Structure of fullerenes and related hollow and planar molecular structures
68.55.ap Fullerenes
68.55.-a Thin film structure and morphology
81.10.-h Methods of crystal growth; physics and chemistry of crystal growth, crystal morphology, and orientation
61.66.-f Structure of specific crystalline solids

Organic electroluminescent diodes

C. W. Tang and S. A. VanSlyke

Appl. Phys. Lett. 51, 913 (1987); http://dx.doi.org/10.1063/1.98799 (3 pages)

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A novel electroluminescent device is constructed using organic materials as the emitting elements. The diode has a double‐layer structure of organic thin films, prepared by vapor deposition. Efficient injection of holes and electrons is provided from an indium‐tin‐oxide anode and an alloyed Mg:Ag cathode. Electron‐hole recombination and green electroluminescent emission are confined near the organic interface region. High external quantum efficiency (1% photon/electron), luminous efficiency (1.5 lm/W), and brightness (>1000 cd/m2) are achievable at a driving voltage below 10 V.
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85.60.Jb Light-emitting devices
72.20.Jv Charge carriers: generation, recombination, lifetime, and trapping
73.61.Cw Elemental semiconductors
73.61.Jc Amorphous semiconductors; glasses
73.61.Le Other inorganic semiconductors
78.60.Fi Electroluminescence
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