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Appl. Phys. Lett. 97, 053109 (2010); http://dx.doi.org/10.1063/1.3467264 (3 pages)

Plasmon assisted single photon emission of CdSe/CdS nanocrystals deposited on random gold film

I. Mallek-Zouari1, S. Buil1, X. Quélin1, B. Mahler2, B. Dubertret2, and J.-P. Hermier1

1Groupe d’Étude de la Matière Condensée, Université de Versailles Saint-Quentin-En-Yvelines, CNRS UMR8635, 45 avenue des États-Unis, 78035 Versailles, France
2Laboratoire de Physique et d’Etude des Matériaux, CNRS UMR8213, ESPCI, 10 rue Vauquelin, 75231 Paris Cedex 05, France

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(Received 13 April 2010; accepted 16 June 2010; published online 4 August 2010)

We have investigated the modifications of the fluorescence properties of single CdSe/CdS nanocrystals deposited close to a semicontinuous gold film. We report a reduction by a factor of ten of the monoexcitonic state decay rate. Due to the structure of the plasmon resonances, the decay depends on the nanocrystal position. Through the detailed study of the collection efficiency, we show that a large fraction of the plasmons are converted in far field single photons. These results demonstrate the great interest of plasmonic devices to control the single photon emission of colloidal nanocrystals.

© 2010 American Institute of Physics

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KEYWORDS and PACS

PACS

  • 78.67.Bf

    Nanocrystals, nanoparticles, and nanoclusters

  • 78.55.Et

    II-VI semiconductors

  • 79.60.-i

    Photoemission and photoelectron spectra

ARTICLE DATA

PUBLICATION DATA

ISSN

0003-6951 (print)  
1077-3118 (online)

For access to fully linked references, you need to log in.
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